CeO2/CNTs复合光催化剂的制备及其对抗生素废水光催化降解研究
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浙江省大学生科技推广项目(2011R428026),浙江省青年基金项目(Q12B030006)


CeO2/CNTs nanotubes and photocataIytic degradation of antibiotics
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Zhejiang Provincial Natural Science Foundation of China under studant Grant No. 2011R428026;Zhejiang Provincial Natural Science Foundation of China under Grant No.Q12B030006;

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    摘要:

    以多壁碳纳米管(MWCNTs)为载体,硝酸锶铵为锶源,采用水热法制备CeO2/CNTs复合管光催化剂.采用场发射扫描电子显微镜(FE.SEM)对碳纳米管负载CeO2前后的形貌进行了的表征;以阿莫西林溶液的降解为目标反应,考察了催化剂的紫外光、可见光(A>420 nm)催化活性.结果表明:所制备的催化剂基本保持了原始MWCNTs的纤维状形貌,二氧化锶在MWCNTs表面分布均匀,MWCNTs增强了污染物在催化剂表面的吸附,提高了对光的吸收和利用,因此所制备的CeO2/MWCNTs复合光催化剂表现出较高的光催化活性.

    Abstract:

    CeO2 coated multiwalled carbon nanotubes(MWCNTs)composite photocatalysts were prepared by hydrothermal method using MWCNTs as a reaction template and ammonium ceric nitrate as a ceric source. The samples were characterized by field emission scanning electron microscopy(SEM). The photodegradation of amoxicillin solution was used to evaluate the photocatalytic activity of the catalyst under UV and visible light irradiation. The results suggest that the CeO2 coated MWCNTs keep tube morphology with the pristine MWCNTs. The prepared CeO2/CNTs photocatalyst shows higher light photocatalytic activity because the MWCNTs increase the adsorption of reactant on the photocatalyst a, which can enhance the absorption and utilization of light.

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卢格斯特,岑立,高翔,等. CeO2/CNTs复合光催化剂的制备及其对抗生素废水光催化降解研究[J]. 科学技术与工程, 2012, 12(24): .
LU Gesite, CEN Li, GAO Xiang, et al. CeO2/CNTs nanotubes and photocataIytic degradation of antibiotics[J]. Science Technology and Engineering,2012,12(24).

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  • 收稿日期:2012-05-08
  • 最后修改日期:2012-05-08
  • 录用日期:2012-05-17
  • 在线发布日期: 2012-07-02
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